Abstract
Human
activities
affect
the
Earth’s
climate
through
modifying
composition
of
atmosphere,
which
then
creates
radiative
forcing
that
drives
change.
The
warming
effect
anthropogenic
greenhouse
gases
has
been
partially
balanced
by
cooling
aerosols.
In
2020,
fuel
regulations
abruptly
reduced
emission
sulfur
dioxide
from
international
shipping
about
80%
and
created
an
inadvertent
geoengineering
termination
shock
with
global
impact.
Here
we
estimate
regulation
leads
to
a
$$+0.2\pm
0.11$$
+0.2±0.11
Wm
−2
averaged
over
ocean.
amount
could
lead
doubling
(or
more)
rate
in
2020
s
compared
since
1980
strong
spatiotemporal
heterogeneity.
is
consistent
recent
observed
2023
expected
make
anomalously
warm.
equivalent
magnitude
measured
increase
planetary
heat
uptake
2020.
also
hemispheric
contrast,
important
implications
for
precipitation
pattern
changes.
Our
result
suggests
marine
cloud
brightening
may
be
viable
method
temporarily
its
unique
challenges
due
inherent
Science Advances,
Journal Year:
2023,
Volume and Issue:
9(37)
Published: Sept. 13, 2023
This
planetary
boundaries
framework
update
finds
that
six
of
the
nine
are
transgressed,
suggesting
Earth
is
now
well
outside
safe
operating
space
for
humanity.
Ocean
acidification
close
to
being
breached,
while
aerosol
loading
regionally
exceeds
boundary.
Stratospheric
ozone
levels
have
slightly
recovered.
The
transgression
level
has
increased
all
earlier
identified
as
overstepped.
As
primary
production
drives
system
biosphere
functions,
human
appropriation
net
proposed
a
control
variable
functional
integrity.
boundary
also
transgressed.
modeling
different
climate
and
land
change
illustrates
these
anthropogenic
impacts
on
must
be
considered
in
systemic
context.
Reviews of Geophysics,
Journal Year:
2020,
Volume and Issue:
58(4)
Published: July 22, 2020
We
assess
evidence
relevant
to
Earth's
equilibrium
climate
sensitivity
per
doubling
of
atmospheric
CO2,
characterized
by
an
effective
S.
This
includes
feedback
process
understanding,
the
historical
record,
and
paleoclimate
record.
An
S
value
lower
than
2
K
is
difficult
reconcile
with
any
three
lines
evidence.
The
amount
cooling
during
Last
Glacial
Maximum
provides
strong
against
values
greater
4.5
K.
Other
in
combination
also
show
that
this
relatively
unlikely.
use
a
Bayesian
approach
produce
probability
density
function
(PDF)
for
given
all
evidence,
including
tests
robustness
difficult-to-quantify
uncertainties
different
priors.
66%
range
2.6–3.9
our
Baseline
calculation
remains
within
2.3–4.5
under
tests;
corresponding
5–95%
ranges
are
2.3–4.7
K,
bounded
2.0–5.7
(although
such
high-confidence
should
be
regarded
more
cautiously).
indicates
stronger
constraint
on
reported
past
assessments,
lifting
low
end
range.
narrowing
occurs
because
agree
judged
largely
independent
confidence
understanding
processes
combining
identify
promising
avenues
further
S,
particular
using
comprehensive
models
address
limitations
traditional
forcing-feedback
paradigm
interpreting
changes.
<p>Aerosol
radiative
forcing
plays
an
important
role
in
the
attribution
of
past
climate
changes,
estimates
future
allowable
carbon
emissions,
and
assessment
potential
geoengineering
solutions.
Substantial
progress
made
over
40
years
observing,
understanding,
modelling
aerosol
processes
helped
quantify
forcing,
but
uncertainties
remain
large.</p><p>In
spring
2018,
under
auspices
World
Climate
Research
Programme's
Grand
Science
Challenge
on
Clouds,
Circulation
Sensitivity,
thirty-six
experts
gathered
to
take
a
fresh
comprehensive
look
at
present
understanding
identify
prospects
for
some
most
pressing
open
questions.
The
outcome
that
meeting
is
review
paper,
Bellouin
et
al.
(2019),
accepted
publication
Reviews
Geophysics.
This
provides
new
range
industrial
era
based
multiple,
traceable
arguable
lines
evidence,
including
approaches,
theoretical
considerations,
observations.
A
substantial
achievement
focus
evidence
rather
than
survey
results
or
expert
judgement,
make
questions
much
more
specific.</p><p>This
talk
will
key
messages
arguments
work
show
promise
improving
quantification
forcing.</p>
Atmospheric chemistry and physics,
Journal Year:
2020,
Volume and Issue:
20(16), P. 9591 - 9618
Published: Aug. 17, 2020
Abstract.
The
effective
radiative
forcing,
which
includes
the
instantaneous
forcing
plus
adjustments
from
atmosphere
and
surface,
has
emerged
as
key
metric
of
evaluating
human
natural
influence
on
climate.
We
evaluate
in
17
contemporary
climate
models
that
are
participating
Coupled
Model
Intercomparison
Project
(CMIP6)
have
contributed
to
Radiative
Forcing
(RFMIP).
Present-day
(2014)
global-mean
anthropogenic
relative
pre-industrial
(1850)
levels
stands
at
2.00
(±0.23)
W
m−2,
comprised
1.81
(±0.09)
m−2
CO2,
1.08
(±
0.21)
other
well-mixed
greenhouse
gases,
−1.01
0.23)
aerosols
−0.09
(±0.13)
land
use
change.
Quoted
uncertainties
1
standard
deviation
across
model
best
estimates,
90
%
confidence
reported
forcings,
due
internal
variability,
is
typically
within
0.1
m−2.
majority
remaining
0.21
likely
be
ozone.
In
most
cases,
largest
contributors
spread
(ERF)
(IRF)
cloud
responses,
particularly
aerosol–cloud
interactions
aerosol
forcing.
As
determined
previous
studies,
cancellation
tropospheric
surface
means
stratospherically
adjusted
approximately
equal
ERF
for
gas
but
not
aerosols,
consequentially,
total.
ranges
−0.63
−1.37
exhibiting
a
less
negative
mean
narrower
range
compared
10
CMIP5
models.
4×CO2
also
narrowed
CMIP6
13
Aerosol
uncorrelated
with
sensitivity.
Therefore,
there
no
evidence
suggest
increasing
sensitivity
models,
related
high-sensitivity
consequence
stronger
present-day
little
modelling
groups
systematically
tuning
or
recreate
observed
historical
warming.
Earth System Dynamics,
Journal Year:
2020,
Volume and Issue:
11(3), P. 737 - 750
Published: Aug. 17, 2020
Abstract.
Climate
sensitivity
to
CO2
remains
the
key
uncertainty
in
projections
of
future
climate
change.
Transient
response
(TCR)
is
metric
temperature
that
most
relevant
warming
next
few
decades
and
contributes
biggest
estimates
carbon
budgets
consistent
with
Paris
targets.
Equilibrium
(ECS)
vital
for
understanding
longer-term
change
stabilisation
In
IPCC
5th
Assessment
Report
(AR5),
stated
“likely”
ranges
(16
%–84
%
confidence)
TCR
(1.0–2.5
K)
ECS
(1.5–4.5
were
broadly
ensemble
CMIP5
Earth
system
models
(ESMs)
available
at
time.
However,
many
latest
CMIP6
ESMs
have
larger
sensitivities,
5
34
having
values
above
2.5
K
an
mean
2.0±0.4
K.
Even
starker,
12
value
4.5
On
face
it,
these
ESM
results
suggest
likely
may
need
revising
upwards,
which
would
cast
further
doubt
on
feasibility
Here
we
show
rather
than
increasing
sensitivity,
help
constrain
range
1.3–2.1
K,
a
central
estimate
1.68
We
reach
this
conclusion
through
emergent
constraint
approach
relates
linearly
global
from
1975
onwards.
This
period
when
signal-to-noise
ratio
net
radiative
forcing
increases
strongly,
so
uncertainties
aerosol
become
progressively
less
problematic.
find
apply
same
method
models.
Our
constraints
are
good
agreement
other
recent
studies
analysed
CMIP
ensembles.
The
relationship
between
post-1975
trend
direct
also
non-linear.
able
derive
1.9–3.4
by
assuming
underlying
based
two-box
energy
balance
model.
Despite
some
methodological
differences;
previously
published
derived
trends
2005.
seem
be
part
growing
consensus
amongst
applied
different
model
ensembles
aspects
record
warming.
Nature Reviews Earth & Environment,
Journal Year:
2020,
Volume and Issue:
1(9), P. 470 - 481
Published: July 29, 2020
Restrictions
to
reduce
human
interaction
have
helped
avoid
greater
suffering
and
death
from
the
COVID-19
pandemic,
but
also
created
socioeconomic
hardship.
This
disruption
is
unprecedented
in
modern
era
of
global
observing
networks,
pervasive
sensing
large-scale
tracking
mobility
behaviour,
creating
a
unique
test
bed
for
understanding
Earth
System.
In
this
Perspective,
we
hypothesize
immediate
long-term
System
responses
along
two
multidisciplinary
cascades:
energy,
emissions,
climate
air
quality;
poverty,
globalization,
food
biodiversity.
While
short-term
impacts
are
dominated
by
direct
effects
arising
reduced
activity,
longer-lasting
likely
result
cascading
economic
recession
on
green
investment
behaviour.
These
offer
opportunity
novel
insight,
particularly
with
careful
deployment
targeted
data
collection,
coordinated
model
experiments
solution-oriented
randomized
controlled
trials,
during
after
pandemic.
The
pandemic
has
caused
substantial
impact.
Perspective
provides
insight
into
environmental
documenting
how
it
offers
an
better
understand
Earth system science data,
Journal Year:
2020,
Volume and Issue:
12(4), P. 3573 - 3620
Published: Dec. 22, 2020
Abstract.
Proven
by
multiple
theoretical
and
practical
studies,
multi-angular
spectral
polarimetry
is
ideal
for
comprehensive
retrieval
of
properties
aerosols.
Furthermore,
a
large
number
advanced
space
polarimeters
have
been
launched
recently
or
planned
to
be
deployed
in
the
coming
few
years
(Dubovik
et
al.,
2019).
Nevertheless,
at
present,
utilization
aerosol
products
from
rather
limited,
due
relatively
small
polarimetric
compared
photometric
observations,
as
well
challenges
making
full
use
extensive
information
content
available
these
complex
observations.
Indeed,
while
recent
several
new
algorithms
developed
provide
enhanced
retrievals
satellite
polarimetry,
value
yet
remains
proven.
In
this
regard,
paper
presents
analysis
obtained
Generalized
Retrieval
Atmosphere
Surface
Properties
(GRASP)
algorithm
POLDER/PARASOL
After
about
decade
development,
GRASP
has
adapted
operational
processing
observations
released.
These
updated
PARASOL/GRASP
are
publicly
(e.g.,
http://www.icare.univ-lille.fr,
last
access:
16
October
2018,
http://www.grasp-open.com/products/,
28
March
2020);
dataset
used
current
study
registered
under
https://doi.org/10.5281/zenodo.3887265
(Chen
2020).
The
objective
comprehensively
evaluate
First,
validation
entire
2005–2013
archive
was
conducted
comparing
ground-based
Aerosol
Robotic
Network
(AERONET)
data.
subjects
optical
depth
(AOD),
absorption
(AAOD)
single-scattering
albedo
(SSA)
six
wavelengths,
Ångström
exponent
(AE),
fine-mode
AOD
(AODF)
coarse-mode
(AODC)
interpolated
reference
wavelength
550
nm.
Second,
an
inter-comparison
with
PARASOL/Operational,
MODIS
Dark
Target
(DT),
Deep
Blue
(DB)
Multi-Angle
Implementation
Atmospheric
Correction
(MAIAC)
year
2008
performed.
Over
land
both
data
validations
inter-comparisons
were
separately
different
surface
types,
discriminated
bins
normalized
difference
vegetation
index
(NDVI):
<
0.2,
0.2
≤
0.4,
0.4
0.6,
≥
0.6.
Three
analyzed:
GRASP/HP
(“High
Precision”),
Optimized
Models.
consistent
but
using
assumptions
modeling
accuracies
atmospheric
radiative
transfer
(RT)
calculations.
Specifically,
when
there
direct
size
distribution
refraction.
When
GRASP/Models,
approximated
mixture
prescribed
components,
each
their
own
fixed
properties,
only
concentrations
those
components
retrieved.
employs
most
accurate
RT
calculations,
GRASP/Optimized
GRASP/Models
optimized
achieve
best
trade-off
between
accuracy
speed.
all
three
options,
underlying
reflectance
retrieved
simultaneously
calculations
performed
“online”
during
retrieval.
All
results
show
solid
quality
characteristics.
retrievals,
however,
provided
products,
e.g.,
(550
nm)
unbiased
highest
correlation
(R
∼
0.92)
fraction
(∼
55.3
%)
satisfying
requirements
Global
Climate
Observing
System
(GCOS)
AERONET
non-negligible
positive
bias
0.07)
low
(<
0.2).
On
other
hand,
detailed
microphysical
characteristics
(AE,
AODF,
AODC,
SSA,
etc.)
correlate
generally
better
than
do
GRASP/Models.
Overall,
demonstrates
high
versus
AERONET.
Evidently,
approach
more
total
AOD,
limited
models
used.
comparative
showed
that,
based
on
against
AERONET,
product
similar
sometimes
higher
products.
good
agreement
over
ocean.
land,
especially
bright
surfaces,
degrades
differences
increase.
characteristics,
such
AE,
AODF
AODC
PARASOL/GRASP,
reliable,
land.
global
robust
agreement,
though
some
patterns
tendencies
observed.
ocean,
PARASOL/Models
MODIS/DT
agree
coefficient
0.92.
lower,
ranging
0.76
0.85.
There
no
significant
offset;
surfaces
tend
values
smaller
moderate
AODs.
Seasonal
means
suggest
that
biomass
burning
loading
central
Africa
dust
Taklamakan
Desert,
less
northern
Sahara.
It
noticeable
also
sites
somewhat
higher,
suggesting
work
rest
globe.
One
potential
reasons
may
general,
rely
climatology
retrievals.
shows
like
POLDER
least
comparable
single-viewing
MODIS-like
imagers.
At
same
time,
AE),
additional
parameters
AAOD
SSA.
Nature Communications,
Journal Year:
2021,
Volume and Issue:
12(1)
Published: Jan. 12, 2021
Uncertainty
in
the
representation
of
biomass
burning
(BB)
aerosol
composition
and
optical
properties
climate
models
contributes
to
a
range
modeled
effects
on
incoming
solar
radiation.
Depending
model,
top-of-the-atmosphere
BB
effect
can
from
cooling
warming.
By
relating
absorption
relative
extinction
carbonaceous
12
observational
datasets
nine
state-of-the-art
Earth
system
models/chemical
transport
models,
we
identify
varying
degrees
overestimation
absorptivity
by
these
models.
Modifications
refractive
index,
size,
mixing
state
improve
Community
Atmosphere
Model
version
5
(CAM5)
agreement
with
observations,
leading
global
change
direct
radiative
-0.07
W
m-2,
regional
changes
-2
m-2
(Africa)
-0.5
(South
America/Temperate).
Our
findings
suggest
that
current
less
warming
than
previously
thought,
largely
due
treatments
state.