Highly flame retardancy, barrier, mechanical and persistent antibacterial polylactic acid film with high-parallel interconnected thousand layered cake architecture DOI
Dongfang Tang, Zuodong Qin, Xiaofang Luo

et al.

International Journal of Biological Macromolecules, Journal Year: 2024, Volume and Issue: 273, P. 132777 - 132777

Published: June 2, 2024

Language: Английский

New insights into balancing wound healing and scarless skin repair DOI Creative Commons
Shengxi Zhou,

Mengbo Xie,

Jingjing Su

et al.

Journal of Tissue Engineering, Journal Year: 2023, Volume and Issue: 14

Published: Jan. 1, 2023

Scars caused by skin injuries after burns, wounds, abrasions and operations have serious physical psychological effects on patients. In recent years, the research of scar free wound repair has been greatly expanded. However, understanding complex mechanisms healing, in which various cells, cytokines mechanical force interact, is critical to developing a treatment that can achieve scarless healing. Therefore, this paper reviews types mechanism formation healing process, current progress dual consideration prevention, some strategies for repair.

Language: Английский

Citations

52

Degradable biomedical elastomers: paving the future of tissue repair and regenerative medicine DOI
Ben Jia,

Heyuan Huang,

Zhicheng Dong

et al.

Chemical Society Reviews, Journal Year: 2024, Volume and Issue: 53(8), P. 4086 - 4153

Published: Jan. 1, 2024

This review critically analyzes degradable biomedical elastomers, focusing on their degradation, synthesis, microstructure, and role in tissue repair. It guides experts balancing degradation with repair for improved applications.

Language: Английский

Citations

49

A human muscle-inspired, high strength, good elastic recoverability, room-temperature self-healing, and recyclable polyurethane elastomer based on dynamic bonds DOI
Shanshan Wang, Xingyu Chen,

Lizhen Guo

et al.

Composites Science and Technology, Journal Year: 2024, Volume and Issue: 248, P. 110457 - 110457

Published: Jan. 21, 2024

Language: Английский

Citations

33

Regulation of Hard Segment Cluster Structures for High‐performance Poly(urethane‐urea) Elastomers DOI Creative Commons
Jianliang Qin, Yifei Chen, Xiwei Guo

et al.

Advanced Science, Journal Year: 2024, Volume and Issue: 11(22)

Published: April 11, 2024

Abstract Elastomers are widely used in daily life; however, the preparation of degradable and recyclable elastomers with high strength, toughness, excellent crack resistance remains a challenging task. In this report, polycaprolactone‐based poly(urethane‐urea) elastomer is presented mechanical properties by optimizing arrangement hard segment clusters. It found that long alkyl chains chain extenders lead to small evenly distributed clusters, which beneficial for improving properties. Together multiple hydrogen bond structure stress‐induced crystallization, obtained exhibits strength 63.3 MPa, an toughness 431 MJ m −3 outstanding fracture energy 489 kJ −2 , while maintaining good recyclability degradability. believed holds great promise various application fields it contributes development sustainable society.

Language: Английский

Citations

21

Degradable, biocompatible, and flexible capacitive pressure sensor for intelligent gait recognition and rehabilitation training DOI
Dedong Guo, Yuanlong Li, Qihui Zhou

et al.

Nano Energy, Journal Year: 2024, Volume and Issue: 127, P. 109750 - 109750

Published: May 18, 2024

Language: Английский

Citations

19

High-Strength and Excellent Self-Healing Polyurethane Elastomer Based on Rigid Chain Segment Reinforcement DOI
Li-Quan Huang,

Hua-Xin Huang,

Ning Yu

et al.

Macromolecules, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 24, 2025

Owing to their extensive application scope, elastomers that combine high strength and excellent self-healing efficiency have always attracted significant attention are still a contradiction. In this study, novel PU elastomer was prepared by combining rigid poly(amic acid) (PAA) chain segments 3,3-dithiodipropionic dihydrazide (DPH) containing sextuple hydrogen-bonding units disulfide bonds. The exhibited tensile of 50.1 MPa toughness 144.2 MJ/m3. PAA serve as framework, significantly enhancing the mechanical elastomer. Meanwhile, DPH with bonds enabled exhibit an 96.1% after 12 h at 80 °C. Additionally, strong reversible cross-linking arrays in endows it strength, ability, recyclability, allowing be recycled hot pressing dissolution.

Language: Английский

Citations

4

A Visible Light-Responsive, Fast Room-Temperature Self- Healing, Mechanically Robust, Antibacterial Waterborne Polyurethane Based on Triple Dynamic Bonds DOI

Yupeng Li,

Yong Jin, Haonan Chen

et al.

ACS Applied Materials & Interfaces, Journal Year: 2025, Volume and Issue: unknown

Published: March 20, 2025

Despite the recent rapid advancements in room-temperature self-healing waterborne polyurethanes, imparting fast ability while concurrently maintaining robust mechanical performance of polyurethanes remains a formidable challenge. Herein, we propose molecular structure design strategy for developing visible light-responsive, self-healing, and antibacterial polyurethane (DMZWPU) containing triple dynamic bonds diselenide bonds, multiple hydrogen Zn(II)–carboxylate coordination bonds. This innovative approach effectively balances tensile stress, fracture toughness, material. Thanks to synergy three resulting DMZWPU film demonstrates stress 40.32 MPa toughness 119.29 MJ/m3, respectively. Furthermore, based on characteristics dual induction trace ethanol light, damaged can recover more than 85% at room temperature within 2 h. These performances outperform those most currently reported self-healable polymers (healing efficiency >80%). Due combined action selenium zinc ions, DWZWPU exhibits excellent properties (sterilization rate 100% 24 h). Finally, emulsion is applied leather finishing processes, results show that coating folding resistance, wear function, as well enhanced water resistance dry friction resistance. In summary, this study provides novel perspective development with high temperature.

Language: Английский

Citations

2

A hyaluronic acid / chitosan composite functionalized hydrogel based on enzyme-catalyzed and Schiff base reaction for promoting wound healing DOI

Jiankang Li,

Jingjing Su,

Jiaheng Liang

et al.

International Journal of Biological Macromolecules, Journal Year: 2023, Volume and Issue: 255, P. 128284 - 128284

Published: Nov. 21, 2023

Language: Английский

Citations

23

Flexible Cages Enable Robust Supramolecular Elastomers DOI
Jing Xu, Mingchao Shao, Xiaoyue Wang

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(16)

Published: Jan. 6, 2024

Abstract Advances in modern industrial technology continue to place stricter demands on engineering polymeric materials, but simultaneously possessing superior strength and toughness remains a daunting challenge. Herein, pioneering flexible cage‐reinforced supramolecular elastomer (CSE) is reported that exhibits superb robustness, tear resistance, anti‐fatigue, shape memory properties, achieved by innovatively introducing organic imide cages (OICs) into networks. Intriguingly, extremely small amounts of OICs make the stronger, significantly improving mechanical (85.0 MPa; ≈10‐fold increase) (418.4 MJ m −3 ; ≈7‐fold increase). Significantly, cooperative effect gradient hydrogen bonds experimentally theoretically demonstrated as nodes, enabling more robust In short, proposed strengthening strategy adding effectively balances inherent conflict between material toughness, prepared CSEs are anticipated be served large‐scale devices such TBMs future.

Language: Английский

Citations

15

Rapidly Gelling, Highly Adhesive, and Mechanically Robust Ionogels for Stretchable and Wireless Electronics DOI
Gang Ge, Yizhou Zhang, Xiao Xiao

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: 34(21)

Published: Jan. 30, 2024

Abstract Stretchable devices function at the biology/electrode interface, depending on excellent conformality between electronic components and nonplanar surfaces. Various polymeric architecture‐based sensing platforms have been extensively explored for physiological signal readout, however, poor interfacial adhesion coupled with low mechanical characteristics lead to easy debonding. Herein, a novel adhesive capable of rapid gelation, strong adhesion, high toughness, achieved through polymerization‐induced phase‐separation strategy is reported. In this design, cosolvent polar polymer serve as amorphous crystalline domains, respectively, performances readily modulable by altering formulation, ultimately reach toughness par elastomers. Remarkably, undergoes sol–gel transition within several seconds, displaying diverse substrates. Capitalizing its enduring wet tissues, wearable device real‐time sweat monitoring during exercise developed. To showcase practical application, portable battery‐free system designed further demonstrate various vertebral postures, aiding regulation activities. This study not only pioneers preparation adhesives but also paves way in era Internet‐of‐Things.

Language: Английский

Citations

12