Advanced Functional Materials,
Journal Year:
2023,
Volume and Issue:
33(24)
Published: April 23, 2023
Abstract
Inherently
tissue‐like
feature
and
multifunctional
property
of
hydrogels
make
themself
excellent
materials
for
flexible
electronics.
However,
conventional
with
insufficient
mechanical
strength
poor
fatigue
resistance
are
damaged
or
lose
service
stability
when
subjected
to
alternating
stress.
Herein,
self‐reinforced
fabricated
from
elaborately
designed
ionic
conductive
after
repetitive
sweat
soak‐dehydration
(SSD)
treatment.
The
tensile
is
improved
930
480
kPa
exhibits
insensitivity
crack
propagation
in
any
direction
6
SSD
treatment
cycles.
In
addition,
the
show
skin
friendliness
compared
commercial
wearable
a
skin‐compatibility
mouse
model.
Bringing
together
those
advantages,
various
skin‐contactable
electronics
utilizing
an
emergency
alarming
system
acute
myocardial
infarction
caused
cardiogenic
shock
also
integrated
that
expected
help
potential
patients
accidents.
ACS Nano,
Journal Year:
2023,
Volume and Issue:
17(6), P. 5211 - 5295
Published: March 9, 2023
Humans
rely
increasingly
on
sensors
to
address
grand
challenges
and
improve
quality
of
life
in
the
era
digitalization
big
data.
For
ubiquitous
sensing,
flexible
are
developed
overcome
limitations
conventional
rigid
counterparts.
Despite
rapid
advancement
bench-side
research
over
last
decade,
market
adoption
remains
limited.
To
ease
expedite
their
deployment,
here,
we
identify
bottlenecks
hindering
maturation
propose
promising
solutions.
We
first
analyze
achieving
satisfactory
sensing
performance
for
real-world
applications
then
summarize
issues
compatible
sensor-biology
interfaces,
followed
by
brief
discussions
powering
connecting
sensor
networks.
Issues
en
route
commercialization
sustainable
growth
sector
also
analyzed,
highlighting
environmental
concerns
emphasizing
nontechnical
such
as
business,
regulatory,
ethical
considerations.
Additionally,
look
at
future
intelligent
sensors.
In
proposing
a
comprehensive
roadmap,
hope
steer
efforts
towards
common
goals
guide
coordinated
development
strategies
from
disparate
communities.
Through
collaborative
efforts,
scientific
breakthroughs
can
be
made
sooner
capitalized
betterment
humanity.
Chemical Reviews,
Journal Year:
2023,
Volume and Issue:
123(16), P. 9982 - 10078
Published: Aug. 5, 2023
Recent
advancements
in
wearable
electronics
offer
seamless
integration
with
the
human
body
for
extracting
various
biophysical
and
biochemical
information
real-time
health
monitoring,
clinical
diagnostics,
augmented
reality.
Enormous
efforts
have
been
dedicated
to
imparting
stretchability/flexibility
softness
electronic
devices
through
materials
science
structural
modifications
that
enable
stable
comfortable
of
these
curvilinear
soft
body.
However,
optical
properties
are
still
early
stages
consideration.
By
incorporating
transparency,
visual
from
interfacing
biological
systems
can
be
preserved
utilized
comprehensive
diagnosis
image
analysis
techniques.
Additionally,
transparency
provides
imperceptibility,
alleviating
reluctance
wear
device
on
exposed
skin.
This
review
discusses
recent
advancement
transparent
a
way
includes
materials,
processing,
devices,
applications.
Materials
discussed
regarding
their
characteristics,
synthesis,
engineering
strategies
property
enhancements.
We
also
examine
bridging
techniques
Building
blocks
systems,
including
sensors,
energy
actuators,
displays,
mechanisms
performances.
Lastly,
we
summarize
potential
applications
conclude
remaining
challenges
prospects.
Materials Horizons,
Journal Year:
2023,
Volume and Issue:
10(8), P. 2800 - 2823
Published: Jan. 1, 2023
Hydrogels
have
been
attracting
increasing
attention
for
application
in
wearable
electronics,
due
to
their
intrinsic
biomimetic
features,
highly
tunable
chemical-physical
properties
(mechanical,
electrical,
etc.),
and
excellent
biocompatibility.
Among
many
proposed
varieties
of
hydrogels,
conductive
polymer-based
hydrogels
(CPHs)
emerged
as
a
promising
candidate
future
sensor
designs,
with
capability
realizing
desired
features
using
different
tuning
strategies
ranging
from
molecular
design
(with
low
length
scale
10-10
m)
micro-structural
configuration
(up
10-2
m).
However,
considerable
challenges
remain
be
overcome,
such
the
limited
strain
sensing
range
mechanical
strength,
signal
loss/instability
caused
by
swelling/deswelling,
significant
hysteresis
signals,
de-hydration
induced
malfunctions,
surface/interfacial
failure
during
manufacturing/processing.
This
review
aims
offer
targeted
scan
recent
advancements
CPH
based
technology,
establishment
dedicated
structure-property
relationships
lab
advanced
manufacturing
routes
potential
scale-up
production.
The
CPHs
sensors
is
also
explored,
suggested
new
research
avenues
prospects
included.
Nano-Micro Letters,
Journal Year:
2022,
Volume and Issue:
14(1)
Published: Sept. 12, 2022
Respiratory
monitoring
plays
a
pivotal
role
in
health
assessment
and
provides
an
important
application
prospect
for
flexible
humidity
sensors.
However,
traditional
sensors
suffer
from
trade-off
between
deformability,
sensitivity,
transparency,
thus
the
development
of
high-performance,
stretchable,
low-cost
is
urgently
needed
as
wearable
electronics.
Here,
ultrasensitive,
highly
deformable,
transparent
are
fabricated
based
on
cost-effective
polyacrylamide-based
double
network
hydrogels.
Concomitantly,
general
method
preparing
hydrogel
films
with
controllable
thickness
proposed
to
boost
sensitivity
hydrogel-based
due
extensively
increased
specific
surface
area,
which
can
be
applied
different
polymer
networks
facilitate
integrated
In
addition,
sustainable
tapioca
rich
hydrophilic
polar
groups
introduced
first
time
second
cross-linked
network,
exhibiting
excellent
water
adsorption
capacity.
Through
synergistic
optimization
structure
composition,
obtained
film
exhibits
ultrahigh
13,462.1%/%RH,
unprecedented.
Moreover,
film-based
sensor
repeatability
ability
work
normally
under
stretching
even
enhanced
sensitivity.
As
proof
concept,
we
integrate
stretchable
specially
designed
wireless
circuit
mask
fabricate
respiratory
interruption
detection
system
Bluetooth
transmission,
enabling
real-time
human
status.
This
strategy
construct
miniaturized
next-generation
devices
various
physiological
signals.
Advanced Materials,
Journal Year:
2022,
Volume and Issue:
35(3)
Published: Nov. 18, 2022
Abstract
Coating
conventional
metallic
electrodes
with
conducting
polymers
has
enabled
the
essential
characteristics
required
for
bioelectronics,
such
as
biocompatibility,
electrical
conductivity,
mechanical
compliance,
and
capacity
structural
chemical
functionalization
of
bioelectrodes.
However,
fragile
interface
between
polymer
electrode
in
wet
physiological
environment
greatly
limits
their
utility
reliability.
Here,
a
general
yet
reliable
strategy
to
seamlessly
hydrogel
coatings
is
established,
featuring
tissue‐like
modulus,
highly‐desirable
electrochemical
properties,
robust
interface,
long‐term
Numerical
modeling
reveals
role
toughening
mechanism,
synergy
covalent
anchorage
long‐chain
polymers,
cross‐linking,
improving
robustness
interface.
Through
vivo
implantation
freely‐moving
mouse
models,
it
shown
that
stable
electrophysiological
recording
can
be
achieved,
while
hydrogel–electrode
remains
during
low‐voltage
stimulation.
This
simple
versatile
design
addresses
long‐standing
technical
challenges
functional
bioelectrode
engineering,
opens
up
new
avenues
next‐generation
diagnostic
brain‐machine
interfaces.
Advanced Functional Materials,
Journal Year:
2022,
Volume and Issue:
32(35)
Published: June 22, 2022
Abstract
Stretchable
conductors
with
the
combination
of
high
elasticity
and
electric
conductivity
have
long
been
pursued
in
soft
electronics.
Liquid
metals
(LMs),
whose
mechanical
properties
match
well
elastomeric
matrix,
successfully
applied
robotics,
electronic
skins
wearable
devices.
But
it
remains
challenging
to
develop
conductive
composite
elastomers
LMs
reversible
adhesion
self‐healing.
Herein,
EGaIn
droplets
are
uniformly
dispersed
into
elastomer,
which
contain
dynamic
disulfide
endow
elastomer
thermal
processability,
recyclability,
wet
adhesion,
With
content
≥40
vol.%,
resultant
shows
1.3
×
104
S
m
−1
,
self‐healing
8.0
h,
strength
up
670
kPa
after
curing
for
2.0
h.
When
serving
as
adhesive,
can
easily
adhere
metal
electrode
light
LED
even
when
stretched
50%.
self‐adhesive
bioelectrode,
also
detect
human
electromyography
signals.
Thus,
not
only
may
this
study
provide
a
new
platform
designing
self‐adhesive,
self‐healing,
liquid
metals,
but
their
promise
facileness
building
damage‐endurable
electronics
applying
human–machine
interfaces.
Advanced Materials,
Journal Year:
2023,
Volume and Issue:
unknown
Published: Aug. 28, 2023
The
rise
of
flexible
and
stretchable
electronics
has
revolutionized
biosensor
techniques
for
probing
biological
systems.
Particularly,
electrochemical
sensors
(FSECSs)
enable
the
in
situ
quantification
numerous
biochemical
molecules
different
entities
owing
to
their
exceptional
sensitivity,
fast
response,
easy
miniaturization.
Over
past
decade,
fabrication
application
FSECSs
have
significantly
progressed.
This
review
highlights
key
developments
electrode
functionalization.
It
delves
into
sensing
various
biomarkers,
including
metabolites,
electrolytes,
signaling
molecules,
neurotransmitters
from
systems,
encompassing
outer
epidermis,
tissues/organs
vitro
vivo,
living
cells.
Finally,
considering
preparation
applications,
current
challenges
future
opportunities
are
discussed.
Journal of Materials Chemistry C,
Journal Year:
2022,
Volume and Issue:
10(14), P. 5380 - 5399
Published: Jan. 1, 2022
This
paper
reviews
the
research
progress
of
conductive
hydrogel
3D
printing
for
flexible
electronics,
with
emphasis
on
methods,
classification
and
materials
synthesis
application
fields.