ACS Applied Materials & Interfaces,
Journal Year:
2019,
Volume and Issue:
11(19), P. 17873 - 17883
Published: April 22, 2019
Soft
composites
are
critical
for
soft
and
flexible
materials
in
energy
harvesting,
actuators,
multifunctional
devices.
One
emerging
approach
to
create
is
through
the
incorporation
of
liquid
metal
(LM)
droplets
such
as
eutectic
gallium
indium
(EGaIn)
highly
deformable
elastomers.
The
microstructure
systems
their
performance;
however,
current
lack
control
particle
size
at
diverse
volume
loadings.
Here,
we
present
a
fabrication
metal-elastomer
with
independently
controllable
tunable
droplet
(100
nm
≤
D
80
μm)
loading
(0
ϕ
80%).
This
achieved
combination
shear
mixing
sonication
concentrated
LM/elastomer
emulsions
subsequent
dilution
homogenization
tune
LM
loading.
These
characterized
utilizing
dielectric
spectroscopy
supported
by
analytical
modeling,
which
shows
high
relative
permittivity
60
(16×
unfilled
elastomer)
composite
=
80%,
low
tan
δ
0.02,
significant
dependence
on
minor
size.
Temperature
response
stability
determined
using
temperature
frequency
sweeps
DSC.
results
demonstrate
wide
phase
(crystallizing
<-85
°C
<
20
μm).
Additionally,
all
electrically
insulating
across
(0.1
Hz-10
MHz)
(-70
100
°C)
ranges
even
up
80%.
We
highlight
benefit
creating
all-soft-matter
stretchable
capacitive
sensors
sensitivity.
further
integrated
into
wearable
sensing
glove
where
identify
different
objects
during
grasping
motions.
work
enables
programmable
robotics
electronics
flexibility
functional
critical.
Annual Review of Materials Research,
Journal Year:
2021,
Volume and Issue:
51(1), P. 381 - 408
Published: May 12, 2021
Gallium
is
a
metal
that
literally
melts
in
your
hand.
It
has
low
toxicity,
near-zero
vapor
pressure,
and
viscosity
similar
to
water.
Despite
possessing
surface
tension
larger
than
any
other
liquid
(near
room
temperature),
gallium
can
form
nonspherical
shapes
due
the
thin,
solid
native
oxide
skin
forms
rapidly
oxygen.
These
properties
enable
new
ways
pattern
metals
(e.g.,
injection
printing)
create
stretchable
soft
devices
with
an
unmatched
combination
of
mechanical
electrical
properties.
The
be
transferred
substrates
manipulated
electrochemically
lower
interfacial
near
zero.
reactivity
drive
wide
range
reactions.
state
makes
it
easy
break
into
particles
for
making
colloids
composites
have
unusual
deformable
nature
filler.
This
review
summarizes
truly
unique
exciting
metals.
Chemical Society Reviews,
Journal Year:
2022,
Volume and Issue:
51(9), P. 3759 - 3793
Published: Jan. 1, 2022
Skin
bioelectronics
are
considered
as
an
ideal
platform
for
personalised
healthcare
because
of
their
unique
characteristics,
such
thinness,
light
weight,
good
biocompatibility,
excellent
mechanical
robustness,
and
great
skin
conformability.
Recent
advances
in
skin-interfaced
have
promoted
various
applications
precision
medicine.
Particularly,
long-term,
continuous
health
monitoring
offer
powerful
analysis
a
broad
spectrum
statuses,
providing
route
to
early
disease
diagnosis
treatment.
In
this
review,
we
discuss
(1)
representative
sensing
devices,
(2)
material
structure
selection,
device
properties,
wireless
technologies
towards
monitoring,
(3)
applications:
acquisition
electrophysiological,
biophysical,
biochemical
signals,
comprehensive
(4)
rational
guidelines
the
design
future
monitoring.
Long-term,
advanced
will
open
unprecedented
opportunities
timely
prevention,
screening,
diagnosis,
treatment,
demonstrating
promise
revolutionise
traditional
medical
practices.
Small,
Journal Year:
2019,
Volume and Issue:
16(12)
Published: Oct. 3, 2019
Abstract
Liquid
metals
are
emerging
as
fluidic
inorganic
materials
in
various
research
fields.
Micro‐
and
nanoparticles
of
Ga
its
alloys
have
received
particular
attention
the
last
decade
due
to
their
non
toxicity
accessibility
ambient
conditions
well
interesting
chemical,
physical,
mechanical,
electrical
properties.
Unique
features
such
a
nature
self‐passivating
oxide
skin
make
Ga‐based
liquid
metal
particles
(LMPs)
distinguishable
from
conventional
context
synthesis
applications.
Here,
recent
advances
bottom‐up
top‐down
synthetic
methods
LMPs,
physicochemical
properties,
applications
summarized.
Finally,
current
status
LMPs
is
highlighted
perspectives
on
future
directions
also
provided.
Small,
Journal Year:
2019,
Volume and Issue:
16(9)
Published: Oct. 1, 2019
Abstract
Motivated
by
the
increasing
demand
of
wearable
and
soft
electronics,
liquid
metal
(LM)‐based
microfluidics
has
been
subjected
to
tremendous
development
in
past
decade,
especially
robotics,
related
fields,
due
unique
advantages
LMs
that
combines
conductivity
deformability
all‐in‐one.
can
be
integrated
as
core
component
into
microfluidic
systems
form
either
droplets/marbles
or
composites
embedded
polymer
materials
with
isotropic
anisotropic
distribution.
The
LM
are
found
have
broad
applications
deformable
antennas,
diodes,
biomedical
sensing
chips,
transient
circuits,
mechanically
adaptive
materials,
etc.
Herein,
recent
progress
LM‐based
their
potential
summarized.
current
challenges
toward
industrial
future
research
orientation
this
field
also
summarized
discussed.
Advanced Materials,
Journal Year:
2019,
Volume and Issue:
32(27)
Published: Oct. 30, 2019
Engineered
nanomaterials
have
been
extensively
employed
as
therapeutics
for
tumor
management.
Meanwhile,
the
complex
niche
along
with
multiple
barriers
at
cellular
level
collectively
hinders
action
of
nanomedicines.
Here,
advanced
strategies
that
hold
promise
overcoming
numerous
biological
facing
nanomedicines
are
summarized.
Starting
from
entry,
methods
promote
tissue
penetration
nanomedicine
and
address
hypoxia
issue
also
highlighted.
Then,
emphasis
is
given
to
significance
both
physical
barriers,
such
membrane-associated
efflux
pumps,
features,
resistance
apoptosis.
The
pros
cons
an
individual
approach
presented.
In
addition,
associated
technical
problems
discussed,
importance
balancing
therapeutic
merits
additional
cost
sophisticated
designs.
Advanced Functional Materials,
Journal Year:
2019,
Volume and Issue:
29(28)
Published: March 28, 2019
Abstract
Patterning
of
liquid
metal
(LM)
is
usually
an
integral
step
toward
its
practical
applications.
However,
the
high
surface
tension
along
with
oxide
makes
direct
patterning
LM
very
challenging.
Existing
techniques
are
designed
for
limited
types
planar
substrates,
which
require
multiple‐step
operation,
delicate
molds
and
masks,
expensive
equipment.
In
this
work,
a
simple,
versatile,
equipment‐free
approach
on
various
substrates
using
magnetic
field
reported.
To
achieve
this,
microparticles
dispersed
into
by
stirring.
When
moving
applied
to
droplet,
aggregated
deform
droplet
continuous
line.
addition,
also
applicable
supermetallophobic
since
significantly
enhances
contact
between
substrate.
Moreover,
remote
manipulation
allows
nonplanar
surfaces,
even
in
narrow
near
closed
space,
impossible
existing
techniques.
A
few
applications
demonstrated
proposed
technique
flexible
electronics
wearable
sensors.
Advanced Healthcare Materials,
Journal Year:
2021,
Volume and Issue:
10(17)
Published: March 16, 2021
Wearable
healthcare
devices
have
garnered
substantial
interest
for
the
realization
of
personal
health
management
by
monitoring
physiological
parameters
individuals.
Attaining
integrity
between
and
biological
interfaces
is
one
greatest
challenges
to
achieving
high-quality
body
information
in
dynamic
conditions.
Liquid
metals,
which
exist
liquid
phase
at
room
temperatures,
are
advanced
intensively
as
conductors
deformable
because
their
excellent
stretchability
self-healing
ability.
The
unique
surface
chemistry
metals
allows
development
various
sensors
wearable
form.
Also,
biocompatibility
verified
through
numerous
biomedical
applications,
holds
immense
potential
uses
on
inside
a
living
body.
Here,
recent
progress
metal-based
electronic
with
respect
featured
properties
processing
technologies
discussed.
Representative
examples
applications
such
biosensors,
neural
interfaces,
soft
interconnection
reviewed.
current
prospects
further
also
discussed,
future
directions
advances
latest
research
explored.
Science Advances,
Journal Year:
2022,
Volume and Issue:
8(13)
Published: March 30, 2022
Intrinsically
stretchable
electronics
represent
an
attractive
platform
for
next-generation
implantable
devices
by
reducing
the
mechanical
mismatch
and
immune
responses
with
biological
tissues.
Despite
extensive
efforts,
soft
electronic
often
exhibit
obvious
trade-off
between
performances
deformability
because
of
limitations
commonly
used
compliant
materials.
Here,
we
introduce
a
scalable
approach
to
create
intrinsically
featuring
deployment
liquid
metal
components
ultrahigh
stretchability
up
400%
tensile
strain
excellent
durability
against
repetitive
deformations.
The
device
architecture
further
shows
long-term
stability
under
physiological
conditions,
conformal
attachments
internal
organs,
low
interfacial
impedance.
Successful
electrophysiological
mapping
on
rapidly
beating
hearts
demonstrates
potential
widespread
applications
in
health
monitoring,
disease
diagnosis,
medical
therapies.
Nature Communications,
Journal Year:
2022,
Volume and Issue:
13(1)
Published: April 21, 2022
Electronic
textiles
capable
of
sensing,
powering,
and
communication
can
be
used
to
non-intrusively
monitor
human
health
during
daily
life.
However,
achieving
these
functionalities
with
clothing
is
challenging
because
limitations
in
the
electronic
performance,
flexibility
robustness
underlying
materials,
which
must
endure
repeated
mechanical,
thermal
chemical
stresses
use.
Here,
we
demonstrate
textile
systems
near-field
powering
created
by
digital
embroidery
liquid
metal
fibers.
Owing
unique
electrical
mechanical
properties
fibers,
conform
body
surfaces
establish
robust
wireless
connectivity
nearby
wearable
or
implantable
devices,
even
strenuous
exercise.
By
transferring
optimized
electromagnetic
patterns
onto
this
way,
a
washable
shirt
that
wirelessly
powered
smartphone
continuously
axillary
temperature
without
interfering
activities.