Abstract
Fine
aerosols,
by
acting
as
cloud
condensation
nuclei,
suppress
rainfall
and
enhance
the
albedo
coverage
of
marine
warm
clouds,
thereby
partly
counteracting
greenhouse-induced
warming.
While
this
is
relatively
well
documented,
co-existing
opposite
effects
giant
nuclei
from
coarse
sea
spray
aerosols
are
poorly
quantified.
Here,
satellite
measurements
show
that
have
comparable
magnitudes
with
sign
to
those
fine
aerosols.
For
fixed
liquid
water
path
increasing
decreased
flux
drop
effective
radius
a
factor
1/4
40%,
respectively.
Conversely,
for
path,
added
enhanced
4
35%,
These
large
contrasting
independent
on
meteorological
conditions.
processes
must
be
fully
incorporated
into
climate
models
faithfully
represent
aerosol
precipitation,
radiative
forcing.
Abstract
Human
activities
affect
the
Earth’s
climate
through
modifying
composition
of
atmosphere,
which
then
creates
radiative
forcing
that
drives
change.
The
warming
effect
anthropogenic
greenhouse
gases
has
been
partially
balanced
by
cooling
aerosols.
In
2020,
fuel
regulations
abruptly
reduced
emission
sulfur
dioxide
from
international
shipping
about
80%
and
created
an
inadvertent
geoengineering
termination
shock
with
global
impact.
Here
we
estimate
regulation
leads
to
a
$$+0.2\pm
0.11$$
+0.2±0.11
Wm
−2
averaged
over
ocean.
amount
could
lead
doubling
(or
more)
rate
in
2020
s
compared
since
1980
strong
spatiotemporal
heterogeneity.
is
consistent
recent
observed
2023
expected
make
anomalously
warm.
equivalent
magnitude
measured
increase
planetary
heat
uptake
2020.
also
hemispheric
contrast,
important
implications
for
precipitation
pattern
changes.
Our
result
suggests
marine
cloud
brightening
may
be
viable
method
temporarily
its
unique
challenges
due
inherent
Geophysical Research Letters,
Journal Year:
2024,
Volume and Issue:
51(15)
Published: Aug. 12, 2024
Abstract
Ships
brighten
low
marine
clouds
from
emissions
of
sulfur
and
aerosols,
resulting
in
visible
“ship
tracks”.
In
2020,
new
shipping
regulations
mandated
an
∼80%
reduction
the
allowed
fuel
content.
Recent
observations
indicate
that
ship
tracks
have
decreased.
Model
simulations
since
2020
induced
a
net
radiative
forcing
+0.12
Wm
−2
.
Analysis
recent
temperature
anomalies
indicates
Northern
Hemisphere
surface
2022–2023
are
correlated
with
observed
cloud
is
spatially
simulated
emission
changes.
Shipping
changes
could
be
accelerating
global
warming.
To
better
constrain
these
estimates,
access
to
position
data
understanding
aerosol
needed.
Understanding
risks
benefits
reductions
difficultly
robust
attribution
highlights
large
uncertainty
attributing
proposed
deliberate
climate
intervention.
npj Climate and Atmospheric Science,
Journal Year:
2024,
Volume and Issue:
7(1)
Published: March 8, 2024
Abstract
Atmospheric
soot
and
organic
particles
from
fossil
fuel
combustion
biomass
burning
modify
Earth’s
climate
through
their
interactions
with
solar
radiation
modifications
of
cloud
properties
by
acting
as
condensation
nuclei
ice
nucleating
particles.
Recent
advancements
in
understanding
individual
microscopic
composition
have
led
to
heightened
interest
microphysical
properties.
This
review
article
provides
an
overview
current
advanced
measurements
offers
insights
into
future
avenues
for
studying
these
To
quantify
morphology
ageing,
fractal
dimension
(
D
f
)
is
a
commonly
employed
quantitative
metric
which
allows
characterize
morphologies
aggregates
relation
ageing
factors
like
internal
mixing
state,
core-shell
structures,
phase,
heterogeneity.
Models
been
developed
incorporate
diversity
metrics
aged
particles,
enabling
assessment
optical
absorption
radiative
forcing
effects.
The
are
complex
they
influenced
particle
sources,
process,
meteorological
conditions.
Furthermore,
soluble
exhibit
diverse
forms
can
engage
liquid–liquid
phase
separation
sulfate
nitrate
components.
Primary
carbonaceous
such
tar
balls
warrant
further
attention
due
strong
light
absorbing
properties,
presence
toxic
constituents,
small
size,
impact
human
health.
Future
research
needs
include
both
atmospheric
modeling
approaches,
focusing
on
changes
the
structures
ensembles,
effects
dynamics
Science Advances,
Journal Year:
2024,
Volume and Issue:
10(12)
Published: March 20, 2024
Marine
cloud
brightening
(MCB)
is
the
deliberate
injection
of
aerosol
particles
into
shallow
marine
clouds
to
increase
their
reflection
solar
radiation
and
reduce
amount
energy
absorbed
by
climate
system.
From
physical
science
perspective,
consensus
a
broad
international
group
scientists
that
viability
MCB
will
ultimately
depend
on
whether
observations
models
can
robustly
assess
scale-up
local-to-global
in
today's
identify
strategies
ensure
an
equitable
geographical
distribution
benefits
risks
associated
with
projected
regional
changes
temperature
precipitation.
To
address
knowledge
gaps
required
societal
implications
MCB,
we
propose
substantial
targeted
program
research-field
laboratory
experiments,
monitoring,
numerical
modeling
across
range
scales.
Nature,
Journal Year:
2022,
Volume and Issue:
610(7930), P. 101 - 106
Published: Oct. 5, 2022
Abstract
Cloud
reflectivity
is
sensitive
to
atmospheric
aerosol
concentrations
because
aerosols
provide
the
condensation
nuclei
on
which
water
condenses
1
.
Increased
due
human
activity
affect
droplet
number
concentration,
liquid
and
cloud
fraction
2
,
but
these
changes
are
subject
large
uncertainties
3
Ship
tracks,
long
lines
of
polluted
clouds
that
visible
in
satellite
images,
one
main
tools
for
quantifying
aerosol–cloud
interactions
4
However,
only
a
small
by
shipping
show
ship
tracks
5,6
Here
we
even
when
no
emissions
change
properties
substantially.
We
develop
new
method
quantify
effect
all
clouds,
showing
increase
more
positive
response
there
tracks.
directly
detect
shipping-induced
property
trade
cumulus
regions
Atlantic,
known
display
almost
Our
results
indicate
previous
studies
were
suffering
from
selection
biases
focusing
imagery.
The
strong
path
find
translates
larger
cooling
climate,
potentially
masking
higher
climate
sensitivity
than
observed
temperature
trends
would
otherwise
suggest.
Proceedings of the National Academy of Sciences,
Journal Year:
2022,
Volume and Issue:
119(41)
Published: Oct. 3, 2022
Global
shipping
accounts
for
13%
of
global
emissions
SO
2
,
which,
once
oxidized
to
sulfate
aerosol,
acts
cool
the
planet
both
directly
by
scattering
sunlight
and
indirectly
increasing
albedo
clouds.
This
cooling
due
aerosol
offsets
some
warming
effect
greenhouse
gasses
is
largest
uncertainty
in
determining
change
Earth’s
radiative
balance
human
activity.
Ship
tracks—the
visible
manifestation
indirect
ship
on
clouds
as
quasi-linear
features—have
long
provided
an
opportunity
quantify
these
effects.
However,
they
have
been
arduous
catalog
typically
studied
only
particular
regions
short
periods
time.
Using
a
machine-learning
algorithm
automate
their
detection
we
more
than
1
million
tracks
provide
climatology.
We
use
this
investigate
stringent
fuel
regulations
introduced
International
Maritime
Organization
2020
prevalence
since
then,
while
accounting
disruption
commerce
caused
COVID-19.
find
marked,
but
clearly
nonlinear,
decline
globally:
An
80%
reduction
x
causes
25%
number
detected.
Proceedings of the National Academy of Sciences,
Journal Year:
2022,
Volume and Issue:
119(46)
Published: Nov. 7, 2022
How
clouds
respond
to
anthropogenic
sulfate
aerosols
is
one
of
the
largest
sources
uncertainty
in
radiative
forcing
climate
over
industrial
era.
This
limits
our
ability
predict
equilibrium
sensitivity
(ECS)-the
global
warming
following
a
doubling
atmospheric
CO2.
Here,
we
use
satellite
observations
quantify
relationships
between
and
low-level
while
carefully
controlling
for
meteorology.
We
then
combine
with
estimates
change
concentration
since
about
1850
constrain
associated
forcing.
estimate
that
cloud-mediated
from
[Formula:
see
text]
W
m-2
ocean
(95%
confidence).
constraint
implies
ECS
likely
2.9
4.5
K
(66%
Our
results
indicate
aerosol
less
uncertain
probably
larger
than
ranges
proposed
by
recent
assessments.
Science Advances,
Journal Year:
2022,
Volume and Issue:
8(29)
Published: July 22, 2022
Ship-tracks
are
produced
by
ship-emitted
aerosols
interacting
with
low
clouds.
Here,
we
apply
deep
learning
models
on
satellite
data
to
produce
the
first
global
climatology
map
of
ship-tracks.
We
show
that
ship-tracks
at
nexus
cloud
physics,
maritime
shipping,
and
fuel
regulation.
Our
captures
major
shipping
lanes
while
missing
others
because
background
conditions.
Ship-track
frequency
is
more
than
10
times
higher
a
previous
survey,
its
interannual
fluctuations
reflect
variations
in
cross-ocean
trade,
activity,
regulations.
Fuel
regulation
can
alter
both
detected
routes
due
cost.
The
2020
regulation,
together
coronavirus
disease
2019
pandemic,
reduced
ship-track
lowest
level
recent
decades
across
globe
may
have
ushered
an
era
frequency.
reduces
aerosol
indirect
forcing
from
ship
emissions
46%
or
between
0.02
0.27
W
m
−2
given
current
estimates.
Atmospheric chemistry and physics,
Journal Year:
2023,
Volume and Issue:
23(14), P. 8259 - 8269
Published: July 25, 2023
Abstract.
New
regulations
from
the
International
Maritime
Organization
(IMO)
limiting
sulfur
emissions
shipping
industry
are
expected
to
have
large
benefits
in
terms
of
public
health
but
may
come
with
an
undesired
side
effect:
acceleration
global
warming
as
climate-cooling
effects
ship
pollution
on
marine
clouds
diminished.
Previous
work
has
found
a
substantial
decrease
detection
tracks
after
IMO
2020
went
into
effect,
changes
large-scale
cloud
properties
been
more
equivocal.
Using
statistical
technique
that
estimates
counterfactual
fields
what
and
radiative
within
isolated
corridor
southeastern
Atlantic
would
absence
shipping,
we
confidently
detect
reduction
magnitude
droplet
effective
radius
decreases
find
evidence
for
brightening
well.
The
instantaneous
forcing
due
aerosol–cloud
interactions
is
estimated
O(1
W
m−2)
corridor,
lending
credence
O(0.1
m−2).
In
addition
their
geophysical
significance,
our
results
also
provide
independent
general
compliance
regulations.