Nature Communications,
Journal Year:
2021,
Volume and Issue:
12(1)
Published: June 15, 2021
Satellite-based
estimates
of
radiative
forcing
by
aerosol-cloud
interactions
(RFaci)
are
consistently
smaller
than
those
from
global
models,
hampering
accurate
projections
future
climate
change.
Here
we
show
that
the
discrepancy
can
be
substantially
reduced
correcting
sampling
biases
induced
inherent
limitations
satellite
measurements,
which
tend
to
artificially
discard
clouds
with
high
cloud
fraction.
Those
missed
exert
a
stronger
cooling
effect,
and
more
sensitive
aerosol
perturbations.
By
accounting
for
biases,
magnitude
RFaci
(from
-0.38
-0.59
W
m-2)
increases
55
%
globally
(133
over
land
33
ocean).
Notably,
further
-1.09
m-2
when
switching
total
optical
depth
(AOD)
fine-mode
AOD
is
better
proxy
CCN
AOD.
In
contrast
previous
weak
satellite-based
RFaci,
improved
one
(especially
land),
resolving
major
difference
models.
Journal of Advances in Modeling Earth Systems,
Journal Year:
2020,
Volume and Issue:
12(8)
Published: May 11, 2020
In
the
atmosphere,
microphysics
refers
to
microscale
processes
that
affect
cloud
and
precipitation
particles
is
a
key
linkage
among
various
components
of
Earth's
atmospheric
water
energy
cycles.
The
representation
microphysical
in
models
continues
pose
major
challenge
leading
uncertainty
numerical
weather
forecasts
climate
simulations.
this
paper,
problem
treating
divided
into
two
parts:
(i)
how
represent
population
particles,
given
impossibility
simulating
all
individually
within
cloud,
(ii)
uncertainties
process
rates
owing
fundamental
gaps
knowledge
physics.
recently
developed
Lagrangian
particle-based
method
advocated
as
way
address
several
conceptual
practical
challenges
representing
particle
populations
using
traditional
bulk
bin
parameterization
schemes.
For
addressing
critical
physics
knowledge,
sustained
investment
for
observational
advances
from
laboratory
experiments,
new
probe
development,
next-generation
instruments
space
needed.
Greater
emphasis
on
work,
which
has
apparently
declined
over
past
decades
relative
other
areas
research,
argued
be
an
essential
ingredient
improving
process-level
understanding.
More
systematic
use
natural
observations
constrain
schemes
also
advocated.
Because
it
generally
difficult
quantify
individual
these
directly,
presents
inverse
can
viewed
standpoint
Bayesian
statistics.
Following
idea,
probabilistic
framework
proposed
combines
elements
statistical
physical
modeling.
Besides
providing
rigorous
constraint
schemes,
there
added
benefit
quantifying
systematically.
Finally,
broader
hierarchical
approach
accelerate
improvements
leveraging
described
paper
related
modeling
(using
schemes),
experimentation,
observations,
methods.
Reviews of Geophysics,
Journal Year:
2018,
Volume and Issue:
56(2), P. 409 - 453
Published: April 17, 2018
The
cloud
droplet
number
concentration
(N
d)
is
of
central
interest
to
improve
the
understanding
physics
and
for
quantifying
effective
radiative
forcing
by
aerosol-cloud
interactions.
Current
standard
satellite
retrievals
do
not
operationally
provide
N
d,
but
it
can
be
inferred
from
optical
depth
(τ
c)
radius
(r
e)
top
temperature.
This
review
summarizes
issues
with
this
approach
quantifies
uncertainties.
A
total
relative
uncertainty
78%
pixel-level
relatively
homogeneous,
optically
thick
unobscured
stratiform
clouds
favorable
viewing
geometry.
even
greater
if
these
conditions
are
met.
For
averages
over
1°
×1°
regions
reduced
54%
assuming
random
errors
instrument
In
contrast,
few
evaluation
studies
against
reference
in
situ
observations
suggest
much
better
accuracy
little
variability
bias.
More
such
required
a
error
characterization.
d
dominated
r
e,
therefore,
improvements
e
would
greatly
quality
retrievals.
Recommendations
made
how
might
achieved.
Some
existing
data
sets
compared
discussed,
best
practices
use
current
passive
instruments
(e.g.,
filtering
criteria)
recommended.
Emerging
alternative
estimates
also
considered.
First,
new
ideas
additional
information
upcoming
spaceborne
second,
approaches
using
high-quality
ground-based
examined.
<p>Aerosol
radiative
forcing
plays
an
important
role
in
the
attribution
of
past
climate
changes,
estimates
future
allowable
carbon
emissions,
and
assessment
potential
geoengineering
solutions.
Substantial
progress
made
over
40
years
observing,
understanding,
modelling
aerosol
processes
helped
quantify
forcing,
but
uncertainties
remain
large.</p><p>In
spring
2018,
under
auspices
World
Climate
Research
Programme's
Grand
Science
Challenge
on
Clouds,
Circulation
Sensitivity,
thirty-six
experts
gathered
to
take
a
fresh
comprehensive
look
at
present
understanding
identify
prospects
for
some
most
pressing
open
questions.
The
outcome
that
meeting
is
review
paper,
Bellouin
et
al.
(2019),
accepted
publication
Reviews
Geophysics.
This
provides
new
range
industrial
era
based
multiple,
traceable
arguable
lines
evidence,
including
approaches,
theoretical
considerations,
observations.
A
substantial
achievement
focus
evidence
rather
than
survey
results
or
expert
judgement,
make
questions
much
more
specific.</p><p>This
talk
will
key
messages
arguments
work
show
promise
improving
quantification
forcing.</p>
Proceedings of the National Academy of Sciences,
Journal Year:
2020,
Volume and Issue:
117(30), P. 17591 - 17598
Published: July 13, 2020
Significance
All
cloud
droplets
on
Earth
form
from
tiny
airborne
particles
known
as
aerosols.
Additional
aerosols
anthropogenic
activity
have
produced
more
but
at
smaller
sizes.
The
smaller,
numerous
in
clouds
do
not
collide
effectively,
therefore
resulting
less
precipitation.
Using
a
combination
of
time-lapse
satellite
imagery
and
air
mass
trajectory
modeling,
we
show
that
can
enhance
fraction
extend
the
lifetime
overcast
fields
primarily
under
stable
atmospheric
conditions
typically
found
off
west
coasts
subtropical
stratocumulus-dominated
regions.
Longer-lived
stronger
cooling
influence
climate
therefore,
need
to
be
correctly
parameterized
models
so
accurate
projections
change
achieved.
Journal of Advances in Modeling Earth Systems,
Journal Year:
2018,
Volume and Issue:
10(11), P. 2786 - 2805
Published: Oct. 15, 2018
Abstract
Aerosol
processes
and,
in
particular,
aerosol‐cloud
interactions
cut
across
the
traditional
physical‐Earth
system
boundary
of
coupled
Earth
models
and
remain
one
key
uncertainties
estimating
anthropogenic
radiative
forcing
climate.
Here
we
calculate
historical
aerosol
effective
(ERF)
HadGEM3‐GA7
climate
model
order
to
assess
suitability
this
for
inclusion
UK
model,
UKESM1.
The
ERF,
calculated
year
2000
relative
1850,
is
large
negative
standard
GA7
leading
an
unrealistic
total
over
twentieth
century.
We
show
how
underlying
assumptions
missing
both
physical
parameterizations
lead
ERF.
A
number
improvements
are
investigated
their
impact
on
These
include
improved
representation
cloud
droplet
spectral
dispersion,
updates
activation
scheme,
black
carbon
optical
properties.
One
largest
contributors
uncertainty
insufficient
knowledge
preindustrial
evaluate
contribution
natural
marine
emissions
dimethyl
sulfide
organic
combination
derived
from
these
studies
weakens
ERF
by
up
50%
original
value
leads
a
more
line
with
assessed
values.
Atmospheric chemistry and physics,
Journal Year:
2019,
Volume and Issue:
19(8), P. 5331 - 5347
Published: April 18, 2019
Abstract.
The
impact
of
aerosols
on
cloud
properties
is
one
the
largest
uncertainties
in
anthropogenic
radiative
forcing
climate.
Significant
progress
has
been
made
constraining
this
using
observations,
but
uncertainty
remains,
particularly
magnitude
rapid
adjustments
to
aerosol
perturbations.
Cloud
liquid
water
path
(LWP)
leading
control
liquid-cloud
albedo,
making
it
important
observationally
constrain
LWP.
Previous
modelling
and
observational
studies
have
shown
that
multiple
processes
play
a
role
determining
LWP
response
perturbations,
effect
can
be
difficult
isolate.
Following
previous
mediating
variables,
work
investigates
use
relationship
between
droplet
number
concentration
(Nd)
for
aerosols.
Using
joint-probability
histograms
account
non-linear
relationship,
finds
broadly
consistent
with
studies.
There
significant
geographical
variation
partly
due
meteorological
factors
(particularly
relative
humidity).
Nd–LWP
negative
majority
regions,
suggesting
aerosol-induced
reductions
could
offset
fraction
instantaneous
from
aerosol–cloud
interactions
(RFaci).
However,
variations
volcanic
shipping
perturbations
indicate
overestimates
causal
Nd
confounding
factors.
weaker
reduction
implied
by
these
“natural
experiments”
means
provides
an
upper
bound
changes
Geoscientific model development,
Journal Year:
2020,
Volume and Issue:
13(12), P. 6383 - 6423
Published: Dec. 21, 2020
Abstract.
We
document
and
evaluate
the
aerosol
schemes
as
implemented
in
physical
Earth
system
models,
Global
Coupled
3.1
configuration
of
Hadley
Centre
Environment
Model
version
3
(HadGEM3-GC3.1)
United
Kingdom
System
(UKESM1),
which
are
contributing
to
sixth
Intercomparison
Project
(CMIP6).
The
simulation
aerosols
present-day
period
historical
ensemble
these
models
is
evaluated
against
a
range
observations.
Updates
microphysics
scheme
documented
well
differences
representation
between
configurations.
additional
interactions
included
UKESM1
lead
emissions
natural
sources
such
dimethyl
sulfide,
mineral
dust
organic
subsequent
evolution
species
model.
also
includes
stratospheric–tropospheric
chemistry
fully
coupled
scheme,
while
GC3.1
employs
simplified
mechanism
driven
by
prescribed
monthly
climatologies
relevant
oxidants.
Overall,
simulated
speciated
mass
concentrations
compare
reasonably
with
Both
capture
negative
trend
sulfate
over
Europe
eastern
States
America
(US)
although
tend
underestimate
both
regions.
Interactive
biogenic
volatile
compounds
an
improved
agreement
US.
Simulated
burdens
similar
despite
2-fold
difference
emissions.
Aerosol
optical
depth
biased
low
source
outflow
regions
but
performs
other
compared
number
satellite
ground-based
retrievals
depth.
generally
within
factor
2
observations,
tending
overestimate
remote
ocean
regions,
apart
from
at
high
latitudes,
Northern
Hemisphere
continents.
Finally,
new
primary
marine
for
first
time.
impact
this
evaluated.
Over
pristine
Southern
Ocean,
it
found
improve
seasonal
cycle
cloud
droplet
relative
underestimations
remain.
This
paper
provides
useful
characterisation
climatology
will
facilitate
understanding
numerous
aerosol–climate
interaction
studies
that
be
conducted
part
CMIP6
beyond.
Journal of Advances in Modeling Earth Systems,
Journal Year:
2019,
Volume and Issue:
11(6), P. 1735 - 1758
Published: May 17, 2019
Abstract
We
analyze
the
atmospheric
processes
that
explain
large
changes
in
radiative
feedbacks
between
two
latest
climate
configurations
of
Hadley
Centre
Global
Environmental
model.
use
a
set
atmosphere‐only
change
simulations
(
amip
and
amip‐p4K
)
to
separate
contributions
differences
feedback
parameter
from
all
model
developments
configurations.
show
are
mostly
driven
by
shortwave
cloud
midlatitudes,
mainly
over
Southern
Ocean.
Two
new
schemes
most
differences:
introduction
aerosol
scheme
development
mixed‐phase
scheme.
Both
reduce
strength
preexisting
negative
midlatitudes.
The
dampens
strong
aerosol‐cloud
interaction,
it
also
suppresses
clear‐sky
feedback.
increases
amount
liquid
water
path
(LWP)
present
day
reduces
increase
LWP
with
warming.
contribute
reducing
warmer
climate.
enhances
strong,
preexisting,
positive
fraction
assess
realism
comparing
present‐day
against
observations
discuss
avenues
could
help
constrain
relevant
processes.
Proceedings of the National Academy of Sciences,
Journal Year:
2020,
Volume and Issue:
117(32), P. 18998 - 19006
Published: July 27, 2020
Significance
Enhancement
of
aerosol
that
can
nucleate
cloud
droplets
increases
the
droplet
number
concentration
and
albedo
clouds.
This
amount
sunlight
reflected
to
space.
Uncertainty
in
how
aerosol−cloud
interactions
over
industrial
period
have
increased
planetary
by
this
mechanism
leads
significant
uncertainty
climate
projections.
Our
work
presents
a
method
for
observationally
constraining
change
due
anthropogenic
emissions:
hemispheric
difference
remotely
sensed
between
pristine
Southern
Ocean
(a
preindustrial
proxy)
polluted
Northern
Hemisphere.
Application
constraint
models
reduces
range
estimated
since
industrialization
suggests
current
underpredict
era.