Atmospheric chemistry and physics,
Journal Year:
2024,
Volume and Issue:
24(12), P. 7331 - 7345
Published: June 27, 2024
Abstract.
General
circulation
models'
(GCMs)
estimates
of
the
liquid
water
path
adjustment
to
anthropogenic
aerosol
emissions
differ
in
sign
from
other
lines
evidence.
This
reduces
confidence
effective
radiative
forcing
climate
by
aerosol–cloud
interactions
(ERFaci).
The
discrepancy
is
thought
stem
part
GCMs'
inability
represent
turbulence–microphysics
cloud-top
entrainment,
a
mechanism
that
leads
reduction
response
an
increase
aerosols.
In
real
atmosphere,
enhanced
entrainment
be
dominant
for
path,
weakening
overall
ERFaci.
We
show
latest
generation
GCMs
includes
models
produce
negative
correlation
between
present-day
cloud
droplet
number
and
key
piece
observational
evidence
supporting
aerosols
one
earlier-generation
could
not
reproduce.
However,
even
with
this
correlation,
preindustrial
values
still
simulated
due
parameterized
precipitation
suppression
mechanism.
adds
correlations
are
necessarily
causal.
investigate
sources
confounding
explain
noncausal
number.
These
results
reminder
assessments
parameters
based
on
multiple
must
carefully
consider
complementary
strengths
different
when
disagree.
<p>Aerosol
radiative
forcing
plays
an
important
role
in
the
attribution
of
past
climate
changes,
estimates
future
allowable
carbon
emissions,
and
assessment
potential
geoengineering
solutions.
Substantial
progress
made
over
40
years
observing,
understanding,
modelling
aerosol
processes
helped
quantify
forcing,
but
uncertainties
remain
large.</p><p>In
spring
2018,
under
auspices
World
Climate
Research
Programme's
Grand
Science
Challenge
on
Clouds,
Circulation
Sensitivity,
thirty-six
experts
gathered
to
take
a
fresh
comprehensive
look
at
present
understanding
identify
prospects
for
some
most
pressing
open
questions.
The
outcome
that
meeting
is
review
paper,
Bellouin
et
al.
(2019),
accepted
publication
Reviews
Geophysics.
This
provides
new
range
industrial
era
based
multiple,
traceable
arguable
lines
evidence,
including
approaches,
theoretical
considerations,
observations.
A
substantial
achievement
focus
evidence
rather
than
survey
results
or
expert
judgement,
make
questions
much
more
specific.</p><p>This
talk
will
key
messages
arguments
work
show
promise
improving
quantification
forcing.</p>
Science,
Journal Year:
2021,
Volume and Issue:
371(6528), P. 485 - 489
Published: Jan. 28, 2021
Making
tracks
The
magnitude
of
the
effect
anthropogenic
aerosols
on
formation
clouds
is
an
important
unknown
about
how
humans
are
affecting
climate.
Studies
stratocumulus
cloud
that
formed
by
ship
exhaust
have
been
used
to
estimate
radiative
impact
this
process,
but
Glassmeier
et
al.
now
show
approach
overestimates
cooling
aerosol
addition
up
200%.
These
findings
underscore
need
quantify
responses
understand
climate
system.
Science
,
issue
p.
485
Proceedings of the National Academy of Sciences,
Journal Year:
2020,
Volume and Issue:
117(32), P. 18998 - 19006
Published: July 27, 2020
Significance
Enhancement
of
aerosol
that
can
nucleate
cloud
droplets
increases
the
droplet
number
concentration
and
albedo
clouds.
This
amount
sunlight
reflected
to
space.
Uncertainty
in
how
aerosol−cloud
interactions
over
industrial
period
have
increased
planetary
by
this
mechanism
leads
significant
uncertainty
climate
projections.
Our
work
presents
a
method
for
observationally
constraining
change
due
anthropogenic
emissions:
hemispheric
difference
remotely
sensed
between
pristine
Southern
Ocean
(a
preindustrial
proxy)
polluted
Northern
Hemisphere.
Application
constraint
models
reduces
range
estimated
since
industrialization
suggests
current
underpredict
era.
Atmospheric chemistry and physics,
Journal Year:
2022,
Volume and Issue:
22(1), P. 641 - 674
Published: Jan. 17, 2022
Aerosol-cloud
interactions
(ACIs)
are
considered
to
be
the
most
uncertain
driver
of
present-day
radiative
forcing
due
human
activities.
The
nonlinearity
cloud-state
changes
aerosol
perturbations
make
it
challenging
attribute
causality
in
observed
relationships
forcing.
Using
correlations
infer
can
when
meteorological
variability
also
drives
both
and
cloud
independently.
Natural
anthropogenic
from
well-defined
sources
provide
"opportunistic
experiments"
(also
known
as
natural
experiments)
investigate
ACI
cases
where
may
more
confidently
inferred.
These
cover
a
wide
range
locations
spatiotemporal
scales,
including
point
such
volcanic
eruptions
or
industrial
sources,
plumes
biomass
burning
forest
fires,
tracks
individual
ships
shipping
corridors.
We
review
different
experimental
conditions
conduct
synthesis
available
satellite
datasets
field
campaigns
place
these
opportunistic
experiments
on
common
footing,
facilitating
new
insights
clearer
understanding
key
uncertainties
Cloud
albedo
strongly
sensitive
background
conditions.
Strong
liquid
water
path
increases
largely
ruled
out
by
averaging
across
experiments.
Opportunistic
have
significantly
improved
process-level
ACI,
but
remains
unclear
how
reliably
found
scaled
global
level,
thus
demonstrating
need
for
deeper
investigation
order
improve
assessments
climate
change.
Geophysical Research Letters,
Journal Year:
2024,
Volume and Issue:
51(15)
Published: Aug. 12, 2024
Abstract
Ships
brighten
low
marine
clouds
from
emissions
of
sulfur
and
aerosols,
resulting
in
visible
“ship
tracks”.
In
2020,
new
shipping
regulations
mandated
an
∼80%
reduction
the
allowed
fuel
content.
Recent
observations
indicate
that
ship
tracks
have
decreased.
Model
simulations
since
2020
induced
a
net
radiative
forcing
+0.12
Wm
−2
.
Analysis
recent
temperature
anomalies
indicates
Northern
Hemisphere
surface
2022–2023
are
correlated
with
observed
cloud
is
spatially
simulated
emission
changes.
Shipping
changes
could
be
accelerating
global
warming.
To
better
constrain
these
estimates,
access
to
position
data
understanding
aerosol
needed.
Understanding
risks
benefits
reductions
difficultly
robust
attribution
highlights
large
uncertainty
attributing
proposed
deliberate
climate
intervention.
Science Advances,
Journal Year:
2024,
Volume and Issue:
10(12)
Published: March 20, 2024
Marine
cloud
brightening
(MCB)
is
the
deliberate
injection
of
aerosol
particles
into
shallow
marine
clouds
to
increase
their
reflection
solar
radiation
and
reduce
amount
energy
absorbed
by
climate
system.
From
physical
science
perspective,
consensus
a
broad
international
group
scientists
that
viability
MCB
will
ultimately
depend
on
whether
observations
models
can
robustly
assess
scale-up
local-to-global
in
today's
identify
strategies
ensure
an
equitable
geographical
distribution
benefits
risks
associated
with
projected
regional
changes
temperature
precipitation.
To
address
knowledge
gaps
required
societal
implications
MCB,
we
propose
substantial
targeted
program
research-field
laboratory
experiments,
monitoring,
numerical
modeling
across
range
scales.
Nature Geoscience,
Journal Year:
2024,
Volume and Issue:
17(5), P. 404 - 410
Published: April 11, 2024
Abstract
With
global
warming
currently
standing
at
approximately
+1.2
°C
since
pre-industrial
times,
climate
change
is
a
pressing
issue.
Marine
cloud
brightening
one
proposed
method
to
tackle
through
injecting
aerosols
into
marine
clouds
enhance
their
reflectivity
and
thereby
planetary
albedo.
However,
because
it
unclear
how
influence
clouds,
especially
cover,
both
projections
the
effectiveness
of
remain
uncertain.
Here
we
use
satellite
observations
volcanic
eruptions
in
Hawaii
quantify
aerosol
fingerprint
on
tropical
clouds.
We
observe
large
enhancement
reflected
sunlight,
mainly
due
an
aerosol-induced
increase
cover.
This
observed
strong
negative
forcing
suggests
that
current
level
driven
by
weaker
net
radiative
than
previously
thought,
arising
from
competing
effects
greenhouse
gases
aerosols.
implies
greater
sensitivity
Earth’s
therefore
larger
response
rising
gas
concentrations
reductions
atmospheric
air
quality
measures.
our
findings
also
indicate
mitigation
via
plausible
most
effective
humid
stable
conditions
tropics
where
solar
radiation
strong.
AGU Advances,
Journal Year:
2020,
Volume and Issue:
1(1)
Published: March 1, 2020
Abstract
The
influence
of
aerosol
particles
on
cloud
reflectivity
remains
one
the
largest
sources
uncertainty
in
our
understanding
anthropogenic
climate
change.
Commercial
shipping
constitutes
a
large
and
concentrated
perturbation
meteorological
regime
where
clouds
have
disproportionally
effect
climate.
Yet,
to
date,
studies
been
unable
detect
climatologically
relevant
radiative
effects
from
shipping,
despite
models
indicating
that
response
should
produce
sizable
negative
forcing
(perturbation
Earth's
energy
balance).
We
attribute
significant
increase
enhanced
droplet
number
concentrations
within
major
corridor
southeast
Atlantic.
Prevailing
winds
constrain
emissions
around
corridor,
which
cuts
through
climatically
important
region
expansive
low
cover.
use
universal
kriging,
classic
geostatistical
method,
estimate
what
properties
would
absence
shipping.
In
morning,
brightening
is
consistent
with
changes
microphysics
alone,
whereas
afternoon,
increases
brightness
microphysical
are
offset
by
decreases
total
amount
water.
calculate
an
effective
Atlantic
approximately
−2
W/m
2
.
Several
years
data
required
identify
clear
signal.
Extrapolating
results
globally,
we
due
aerosol‐cloud
interactions
−1.0
(95%
confidence
interval:
−1.6
−0.4
).
unique
setup
could
be
ideal
test
for
representation
models.