Acta Materialia,
Journal Year:
2024,
Volume and Issue:
276, P. 120153 - 120153
Published: July 4, 2024
Superconducting
quantum
circuits
(SQC)
are
one
of
the
most
promising
hardware
platforms
for
computing,
yet
their
performance
is
currently
limited
by
presence
various
structural
defects
inside
circuit's
structure.
Despite
impressive
progress
in
past
decade,
a
precise
understanding
origin
these
from
fabrication
processes
and
impact
on
coherence
still
lacking.
In
this
study,
we
performed
comprehensive
investigation
microstructure,
superconductivity,
resonator
quality
factor
Nb
films
deposited
high-power
impulse
magnetron
sputtering
(HiPIMS)
direct
current
(DC)
sputtering.
A
suite
characterization
techniques,
including
electron
microscopy
with
spectroscopy,
secondary
ion
mass
spectrometry,
magneto-optical
microscopy,
pump-probe
reflectivity
spectroscopy
used.
We
reveal
that
niobium
(Nb)
resonators
fabricated
using
HiPIMS
exhibit
smaller
average
grain
size,
thicker
surface
oxide
larger
thickness
variations
(rougher
surface),
amorphous
Nb/Si
interface
layer
compared
to
samples
DC
identified
oxides
(mainly
located
at
along
boundaries)
Nb-Si
layers
(at
interface)
major
potential
sources
two-level
system
(TLS),
while
off-stochiometric
suboxides
close
surface,
crystalline
(i.e.,
dislocations
boundary,
point
introduced
during
deposition)
main
contributors
non-TLS
sources.
Our
findings
clarify
relationship
between
different
loss
mechanisms,
highlighting
importance
material
microstructure
control
optimization
SQC.
Nature Communications,
Journal Year:
2024,
Volume and Issue:
15(1)
Published: May 1, 2024
The
performance
of
superconducting
quantum
circuits
for
computing
has
advanced
tremendously
in
recent
decades;
however,
a
comprehensive
understanding
relaxation
mechanisms
does
not
yet
exist.
In
this
work,
we
utilize
multimode
approach
to
characterizing
energy
losses
circuits,
with
the
goals
predicting
device
and
improving
coherence
through
materials,
process,
circuit
design
optimization.
Using
approach,
measure
significant
reductions
surface
bulk
dielectric
by
employing
tantalum-based
materials
platform
annealed
sapphire
substrates.
With
knowledge
predict
times
aluminum-
transmon
qubits,
find
that
they
are
consistent
experimental
results.
We
additionally
optimize
geometry
maximize
within
coaxial
tunnel
architecture,
realize
on-chip
memories
single-photon
Ramsey
2.0
-
2.7
ms,
limited
their
1.0
1.4
ms.
These
results
demonstrate
an
advancement
towards
more
modular
compact
architecture
bosonic
qubits
reproducibly
high
coherence.
Physical Review Applied,
Journal Year:
2024,
Volume and Issue:
21(2)
Published: Feb. 23, 2024
Niobium
offers
the
benefit
of
increased
operating
temperatures
and
frequencies
for
Josephson
junctions,
which
are
core
component
superconducting
devices.
However
existing
niobium
processes
limited
by
more
complicated
fabrication
methods
higher
losses
than
now-standard
aluminum
junctions.
Combining
recent
trilayer
advancements,
to
remove
lossy
dielectrics
modern
qubit
design,
we
revisit
junctions
fabricate
all-niobium
transmons
using
only
optical
lithography.
We
characterize
devices
in
microwave
domain,
measuring
coherence
times
up
$62~\mu$s
an
average
quality
factor
above
$10^5$:
much
closer
state-of-the-art
aluminum-junction
find
gap
energy
also
results
reduced
quasiparticle
sensitivity
$0.16~$K,
where
junction
performance
deteriorates.
Our
process
is
readily
applied
standard
optical-based
foundry
processes,
opening
new
avenues
direct
integration
scalability,
paves
way
higher-temperature
higher-frequency
quantum
Physical Review Applied,
Journal Year:
2023,
Volume and Issue:
20(1)
Published: July 26, 2023
Resonator
measurements
are
a
simple
but
powerful
tool
to
characterize
material's
microwave
response.
The
losses
of
resonant
mode
quantified
by
its
internal
quality
factor
${Q}_{\mathrm{i}}$,
which
can
be
extracted
from
the
scattering
coefficient
in
reflection
or
transmission
measurement.
Here
we
show
that
systematic
error
on
${Q}_{\mathrm{i}}$
arises
Fano
interference
signal
with
background
path.
Limited
knowledge
interfering
paths
given
setup
translates
into
range
uncertainty
for
increases
coupling
coefficient.
We
experimentally
illustrate
relevance
typical
resonator
and
associated
pitfalls
encountered
extracting
${Q}_{\mathrm{i}}$.
On
other
hand,
also
how
utilize
eliminate
error.
Physical Review Research,
Journal Year:
2023,
Volume and Issue:
5(4)
Published: Oct. 2, 2023
The
reproducibility
of
qubit
parameters
is
a
challenge
for
scaling
up
superconducting
quantum
processors.
Signal
cross
talk
imposes
constraints
on
the
frequency
separation
between
neighboring
qubits.
uncertainty
transmon
qubits
arising
from
fabrication
process
attributed
to
deviations
in
Josephson
junction
area,
tunnel
barrier
thickness,
and
shunt
capacitor.
We
decrease
sensitivity
these
variations
by
fabricating
larger
junctions
reduce
wafer-level
standard
deviation
resistance
down
2%.
characterize
32
identical
demonstrate
frequencies
with
40
MHz
(i.e.,
1%)
quality
factors
exceeding
2
million.
perform
two-level-system
(TLS)
spectroscopy
observe
no
significant
increase
number
TLSs
causing
relaxation.
further
show
simulation
that
our
parametric-gate
architecture,
accounting
only
errors
caused
frequency,
we
can
scale
100
an
average
three
collisions
quantum-gate
transition
frequencies,
assuming
$2%$
$99.9%$
target
gate
fidelity.
Superconductor Science and Technology,
Journal Year:
2023,
Volume and Issue:
36(6), P. 063002 - 063002
Published: March 7, 2023
Performance
of
superconducting
resonators,
particularly
cavities
for
particle
accelerators
and
micro
thin
film
resonators
quantum
computations
photon
detectors
has
been
improved
substantially
by
recent
materials
treatments
technological
advances.
As
a
result,
the
niobium
have
reached
quality
factors
$Q\sim
10^{11}$
at
1-2
GHz
1.5
K
breakdown
radio-frequency
(rf)
fields
$H$
close
to
dc
superheating
field
Meissner
state.
These
advances
raise
question
whether
state-of-the-art
are
fundamental
limits,
what
these
limits
actually
are,
extent
$Q$
can
be
pushed
nano
structuring
impurity
management.
issues
also
relevant
many
applications
using
high-Q
including
single-photon
circuits.
This
topical
review
outlines
basic
physical
mechanisms
rf
nonlinear
surface
impedance
controlled
quasiparticles,
dielectric
losses
trapped
vortices,
as
well
dynamic
limit
Sections
cover
ways
engineering
an
optimum
quasiparticle
density
states
superfluid
reduce
kinetic
inductance
pairbreaking
related
magnetic
impurities,
currents,
proximity-coupled
metallic
layers
surface.
A
section
focuses
on
residual
resistance
which
dominates
ultra
low
temperatures.
Microwave
vortices
their
reduction
optimizing
concentration
impurities
pinning
potential
discussed.
ACS Nano,
Journal Year:
2024,
Volume and Issue:
unknown
Published: July 21, 2024
Improving
the
qubit's
lifetime
(T1)
is
crucial
for
fault-tolerant
quantum
computing.
Recent
advancements
have
shown
that
replacing
niobium
(Nb)
with
tantalum
(Ta)
as
base
metal
significantly
increases
T1,
likely
due
to
a
less
lossy
native
surface
oxide.
However,
understanding
formation
mechanism
and
nature
of
both
oxides
still
limited.
Using
aberration-corrected
transmission
electron
microscopy
energy
loss
spectroscopy,
we
found
Ta
oxide
has
fewer
suboxides
than
Nb
We
observed
an
abrupt
oxidation
state
transition
from
Ta2O5
Ta,
opposed
gradual
shift
Nb2O5,
NbO2,
NbO
Nb,
consistent
thermodynamic
modeling.
Additionally,
amorphous
exhibits
closer-to-crystalline
bonding
potentially
hindering
H
atomic
diffusion
toward
oxide/metal
interface.
Finally,
propose
arising
between
two
states
within
distorted
octahedron
in
structure,
causing
two-level
system
loss.
Our
findings
offer
deeper
differences
oxides,
providing
valuable
insights
advancing
superconducting
qubits
through
engineering.
Advanced Functional Materials,
Journal Year:
2024,
Volume and Issue:
34(36)
Published: April 10, 2024
Superconducting
Nb
thin
films
have
recently
attracted
significant
attention
due
to
their
utility
for
quantum
information
technologies.
In
the
processing
of
films,
fluoride-based
chemical
etchants
are
commonly
used
remove
surface
oxides
that
known
affect
superconducting
devices
adversely.
However,
these
same
can
also
introduce
hydrogen
form
hydrides,
potentially
negatively
impacting
microwave
loss
performance.
Here,
we
present
comprehensive
materials
characterization
hydrides
formed
in
as
a
function
fluoride
treatments.
particular,
secondary-ion
mass
spectrometry,
X-ray
scattering,
and
transmission
electron
microscopy
reveal
spatial
distribution
phase
transformation
hydrides.
The
rate
hydride
formation
is
determined
by
solution
acidity
etch
Nb2O5,
which
acts
diffusion
barrier
into
Nb.
resulting
detrimental
properties
lead
increased
power-independent
coplanar
waveguide
resonators.
do
not
correlate
with
two-level
system
or
device
aging
mechanisms.
Overall,
this
work
provides
insight
role
loss,
thus
guiding
ongoing
efforts
maximize
coherence
time
devices.
APL Materials,
Journal Year:
2024,
Volume and Issue:
12(2)
Published: Feb. 1, 2024
Tantalum
thin
films
sputtered
on
unheated
silicon
substrates
are
characterized
with
microwaves
at
around
10
GHz
in
a
mK
environment.
We
show
that
the
phase
of
tantalum
body-centered
cubic
lattice
(α-Ta)
can
be
grown
selectively
by
depositing
niobium
buffer
layer
prior
to
film.
The
physical
properties
films,
such
as
superconducting
transition
temperature
and
crystallinity,
change
markedly
addition
layer.
Coplanar
waveguide
resonators
based
composite
film
exhibit
significantly
enhanced
internal
quality
factors
compared
without
factor
approaches
2
×
107
large-photon-number
limit.
While
decreases
single-photon
level
owing
two-level
system
(TLS)
loss,
we
have
deduced
one
causes
TLS
loss
is
amorphous
film–substrate
interface,
which
originates
from
substrate
cleaning
before
deposition
rather
than
itself.
dependence
shows
marked
rise
below
200
mK,
suggesting
presence
TLS–TLS
interactions.
present
low-loss
deposited
heating
thus
various
potential
applications
quantum
electronics.